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Tin Selenide Thin Films Prepared Through Combination of Chemical Precipitation and Vacuum Evaporation Technique

Z. Zainal ¹, S. Nagalingam ¹, A. Kassim ¹, M.Z. Hussein ¹, W.M.M. Yunus ^2
1Department of Chemistry, University Putra Malaysia, Selangor, Malaysia
²Department of Physics, University Putra Malaysia, Selangor, Malaysia

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New Trends in the Investigations of Macrocyclic Magnets

J. Mroziński¹, A. Tomkiewicz¹, M. Nahorska¹, A. Skorupa¹, B. Korybut-Daszkiewicz^2
1Faculty of Chemistry, University of Wrocław, Poland
²Institute of Organic Chemistry, Polish Academy of Sciences, Warszawa, Poland

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Thiolato-bridged Copper Complexes with N,N,S-tridentate Ligands

T. Kotera¹, A. Fujita¹, M. Mikuriya¹, M. Handa^2
1Department of Chemistry, School of Science and Technology, Kwansei Gakuin University, Japan
²Department of Material Science, Interdisciplinary Faculty of Science and Engineering, Shimane University, Japan

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Structural Effects on Magnetism of Pyridyl Nitroxide Complexes of Ruthenium(II, III) Pivalate Dimers

M. Handa¹, Y. Sayama², M. Mikuriya², I. Hiromitsu¹, K. Kasuga^1
1Department of Material Science, Interdisciplinary Faculty of Science and Engineering, Shimane University, Japan
²Department of Chemistry, School of Science and Technology, Kwansei Gakuin University, Japan

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Metal Complexes Immobilised In/On Porous Matrices - Possible Enzyme Mimics

I. Labádi¹, I. Szilágyi¹, N.I. Jakab², K. Hernádi³, I. Pálinkó^2
1Department of Inorganic and Analytical Chemistry, University of Szeged, Hungary
²Department of Organic Chemistry, University of Szeged, Hungary
³Department of Applied and Environmental Chemistry, University of Szeged, Hungary

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Intramolecular Electron Transfer on the Vibrational Timescale in Mixed Valence Ruthenium Clusters

N. Imai, T. Hamaguchi, T. Yamaguchi, T. Ito
Department of Chemistry, Graduate School of Science, Tohoku University, Sendai, Japan

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Copper(I) Complexes as Potential CVD Precursors - Studies in the Liquid State and Gas Phase

I. Szymańska, R. Kucharek, E. Szłyk
Department of Chemistry, Nicolaus Copernicus University, Toruń, Poland

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Spin Crossover in a Supramolecular FeII-FeIII System

H. Ohta¹, Y. Sunatsuki¹, Y. Ikuta², N. Matsumoto², S. Iijima³, H. Akashi⁴, T. Kambe⁵, M. Kojima1
¹Department of Chemistry, Faculty of Science, Okayama University,Tsushima, Japan
²Department of Chemistry, Faculty of Science, Kumamoto University, Japan
³National Institute of Advanced Industrial Science and Technology, Japan
⁴Research Institute of Natural Sciences, Okayama University of Science, Ridai-cho, Japan
⁵Department of Physics, Faculty of Science, Okayama University, Tsushima, Japan

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Spin-entropy Driven Charge Transfer Phase Transition in Iron Mixed-Valence System

N. Kojima, M. Itoi, Y. Ono, M. Okubo, M. Enmoto
Graduate School of Arts and Sciences, The University of Tokyo, Japan

Abstract

We have synthesized iron mixed-valence complexes, (n-C_nH_2n+1)4N[Fe^IIFe^IIIX₃] (X = mto(C₂O₃S), dto(C₂O₂S₂), tto(C₂OS₃)) and have investigated their physical properties by means of ⁵⁷Fe Mössbauer spectroscopy, magnetic susceptibility and electrical resistivity measurements. From the analysis of ⁵⁷Fe Mössbauer spectra, magnetic susceptibility and electrical resistivity, we have discovered a new type of first order phase transition around 120°K for (n-C_nH_2n+1)4N[Fe^IIFe^III(dto)₃](n = 3, 4), where the charge transfer transition between Fe^{II and FeIII occurs reversibly. In the higher temperature phase, the FeIII (S = 1/2) and FeII (S = 2) sites are coordinated by six S atoms and six O atoms, respectively. In the lower temperature phase, on the other hand, the FeIII (S = 5/2) and FeII (S = 0) sites are coordinated by six O atoms and six S atoms, respectively. Moreover, we have found the ferromagnetic phase transition in this system. The ferromagnetic order is induced by the charge transfer interaction between the FeIII and FeII sites. Moreover, we propose various multifunctional properties for (n-C_nH_2n+1)4N[FeIIFeIII(mto)₃] and (n-C_nH_2n+1)4N[FeIIFeIII(tto)₃].}

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Zeta Potential and Doping in Polyaniline Dispersions

D.W.O. de Medeiros¹, D.S. dos Santos², T.N.C. Dantas¹, M.R. Pereira¹, A. Giacometti³, J.L.C. Fonseca^1
1Departamento de Química Universidade Federal do Rio Grande do Norte Lagoa Nova, Natal, Brazil
²Grupo de Polímeros ,,Prof. Bernhard Gross''Instituto de Física de Sao Carlos, Universidade de Sao Paulo, Brazil
³Faculdade de Ciencias e Tecnologia de Presidente Prudente Universidade Estadual Paulista, Brazil

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The Study of the Spin Transition Process in Na[Fe(Th-Sa)₂] by Electron Paramagnetic Resonance

Yu.V. Yablokov¹, V.V. Zelentsov², M. Augustyniak-Jabłokow¹, A. Krupska¹, J. Mroziński^3
1Institute of Molecular Physics PAS, Poznań, Poland
²Moscow Physical Technical Institute, Russia
³Faculty of Chemistry University of Wrocław, Poland

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